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By Gould R.F. (ed.)

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Nor. Skogind. 1957, 11, 284. , 1989. , /. Appl. Polym. Sei. 1985, 30, 3779-3790. , Polymer 1987, 28, 1265-1270. , Acta Polym. 1990, 41, 131-137. , Acta Polym. 1992, 43, 270274. , Papier (Darmstadt) 1994, 48, 739-748. , Science 1954, 779, 80-82. , /. Am. Chem. Soc. 1948, 70, 1107. , Biopolymers 1974,13, 1975-2001. H. ), New York: John Wiley, 1989, pp. V117-V170. , /. Polym. ScL 1958, 28, 432. D. Thesis, Technical University of Dresden 1985. , /. Cell. Biol. 1966, 29, 181-197. , Polymer 1987, 28, 1271-1276.

This spatial chain conformation of crystalline cellulose I and II is adequately represented by a 1,2 helix (Zugenmaier, 1989; Gardner and Blackwell, 1974; Kolpak and Blackwell, 1976). , 1987). Larger deviations from the two-fold helix are discussed for regions of low order in the cellulose solid state structure. 2 The supramolecular structure As described before the cellulose chains have a strong tendency to aggregate to highly ordered structural entities due to their chemical constitution and their spatial conformation.

6 8000-400000 a The term 'porosity' denotes the total percentage of pores including the large ones (>1000nm). Due to the pore and void system, the total surface area of cellulose fibers exceeds by far the geometrical outer surface. The so-called inner surface area is a decisive factor with regard to accessibility and reactivity in dissolution and derivatization processes of the polymer. The data published on inner surface area cover a wide range, from below 1 to about 1000 m^/g, depending on origin and history of the sample, as well as on the procedure of determination.

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